Short-Time Glassy Dynamics in Viscous Protein Solutions with Competing Interactions

Author(s)Godfrin, P. Douglas
Author(s)Hudson, Steven D.
Author(s)Hong, Kunlun
Author(s)Porcar, Lionel
Author(s)Falus, Peter
Author(s)Wagner, Norman J.
Author(s)Liu, Yun
Ordered AuthorP. Douglas Godfrin, Steven D. Hudson, Kunlun Hong, Lionel Porcar, Peter Falus, Norman J. Wagner, and Yun Liu
UD AuthorGodfrin, P. Douglasen_US
UD AuthorWagner, Norman J.en_US
UD AuthorLiu, Yunen_US
Date Accessioned2016-04-07T14:42:54Z
Date Available2016-04-07T14:42:54Z
Copyright DateCopyright © 2015 American Physical Society.en_US
Publication Date2015-11-24
DescriptionPublisher's PDFen_US
AbstractThe glass transition of colloidal dispersions interacting with both a short-ranged attraction and long-ranged repulsion is studied using highly purified lysozyme solutions. Newtonian liquid behavior is observed at all conditions while measurements of the dynamics in the short-time limit show features typical of glassy colloidal systems at high protein concentrations. This interesting behavior is due to the competition of the attraction and repulsion that produces a heterogeneous microstructure only at intermediate range length scales. The results demonstrate that theories for the macroscopic properties of systems with competing interactions need to include intermediate range order.en_US
DepartmentUniversity of Delaware. Department of Chemical & Biomolecular Engineering.en_US
CitationGodfrin, P. Douglas, et al. "Short-Time Glassy Dynamics in Viscous Protein Solutions with Competing Interactions." Physical review letters 115.22 (2015): 228302.en_US
DOIDOI: 10.1103/PhysRevLett.115.228302en_US
ISSN0031-9007 ; e- 1079-7114en_US
URLhttp://udspace.udel.edu/handle/19716/17582
Languageen_USen_US
PublisherAmerican Physical Societyen_US
dc.rightsArticle is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.en_US
dc.sourcePhysical Review Lettersen_US
dc.source.urihttp://journals.aps.org/prl/en_US
TitleShort-Time Glassy Dynamics in Viscous Protein Solutions with Competing Interactionsen_US
TypeArticleen_US
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